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  • This dataset contains model output data on sulphate aerosols, aerosol size distributions and radiative fluxes produced from experiments that used different values of cloud-water pH. The composition-climate model HadGEM3-UKCA was run over the period 1970 to 2009 to investigate the effect of temporal changes in cloud-water pH on sulphate aerosol formation and the subsequent impact on climate. HadGEM3-UKCA is the climate model configuration of the Met Office Unified Model (UM). Vn7.3 of the UM was used in this study and included a branch to the CLOMAP-Mode aerosol scheme. Model simulations were conducted at a global resolution of 1.875° x 1.25°.